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New organic reactivity has often been discovered by happenstance. Several recent research efforts have attempted to leverage this to discover new reactions. In this Review, we attempt to
unify reported approaches to reaction discovery on the basis of the practical and strategic principles applied. We concentrate on approaches to reaction discovery as opposed to reaction
development, though conceptually groundbreaking approaches to identifying efficient catalyst systems are also considered. Finally, we provide a critical overview of the utility and
application of the reported methods from the perspective of a synthetic chemist, and consider the future of high-throughput screening in reaction discovery.
We are grateful to the European Research Council (ERC) under the European Community's Seventh Framework Program (FP7 2007-2013)/ERC grant agreement no 25936, and the DFG (Leibniz award) for
generous financial support.
Organisch-Chemisches Institut, Westfälische Wilhelms-Universität Münster, Corrensstrasse 40, Münster, 48149, Germany
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